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Directly photoexcited Dirac and Weyl fermions in ZrSiS and NbAs
C.P. Weber, L.M. Schoop, S.S.P. Parkin, R.C. Newby, A. Nateprov, B. Lotsch, , J.M. Kim, K.M. Dani, H.A. BechtelShow More
Published in American Institute of Physics Inc.
2018
Volume: 113
   
Issue: 22
Abstract
We report ultrafast optical measurements of the Dirac line-node semimetal ZrSiS and the Weyl semimetal NbAs, using mid-infrared pump photons from 86 meV to 500 meV to directly excite Dirac and Weyl fermions within the linearly dispersing bands. In NbAs, the photoexcited Weyl fermions initially form a non-thermal distribution, signified by a brief spike in the differential reflectivity whose sign is controlled by the relative energy of the pump and probe photons. In ZrSiS, electron-electron scattering rapidly thermalizes the electrons, and the spike is not observed. Subsequently, hot carriers in both materials cool within a few picoseconds. This cooling, as seen in the two materials' differential reflectivity, differs in sign, shape, and timescale. Nonetheless, we find that it may be described in a simple model of thermal electrons, without free parameters. The electronic cooling in ZrSiS is particularly fast, which may make the material useful for optoelectronic applications. © 2018 Author(s).
About the journal
JournalData powered by TypesetApplied Physics Letters
PublisherData powered by TypesetAmerican Institute of Physics Inc.
ISSN00036951