An organophotoredox-catalyzed reduction/addition/oxidation cascade of N-protected maleimides and N-(acyloxy)phthalimides is documented. The mild and efficient redox-neutral process involves the hitherto unknown Giese-type addition of aryloxy-alkyl radicals on N-protected maleimides and a successive oxidation allowing an overall Z-alkenylation of the N-substituted pyrrolidine-2,5-dione motif through a formal translocation of the maleimide double bond. © the Partner Organisations.

Sandip Murarka

Department of Chemistry

IIT Jodhpur

S. Das

S.K. Parida

T. Mandal

S.K. Hota

L. Roy

S. De Sarkar

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Organic Chemistry Frontiers

An organophotoredox-catalyzed redox-neutral cascade involving: N -(acyloxy)phthalimides and maleimides

Journal	Data powered by TypesetOrganic Chemistry Frontiers
Publisher	Data powered by TypesetRoyal Society of Chemistry
ISSN	20524110